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The prefered tautomer(s) of hydroxycyclotriphosphazatrienes and prototropic exchange in solution have been established by 31P n.m.r. spectroscopy, thus confirming predictions deduced from basicity calculations; the X-ray structure of N3P3Ph2(OMe)3OH shows that it exists as the hydrogen-bonded dimer of the oxophosphazadiene tautomer in which a proton is adjacent to the PPh2 group.
K. S. Dhathathreyan, S. S. Krishnamurthy, A. R. V. Murthy, T. S. Cameron, C. Chan, R. A. Shaw and M. Woods, J. Chem. Soc., Chem. Commun., 1980, 231 DOI: 10.1039/C39800000231
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